Express estimation of soil pollution density by planting isotopes of chernobyl origin
DOI:
https://doi.org/10.31548/dopovidi2022.04.001Keywords:
density of radioactive contamination, 90Sr, 238Pu, 239, 240Pu, Chernobyl accidentAbstract
The article considers an approach of finding a rapid estimate of soil contamination density of plutonium isotopes in a radiological survey of agricultural lands on the south-western trace of Chernobyl radioactive fallout outside the Chernobyl Exclusion Zone. An algorithm based on a linear correlation between values of 90Sr and 238,239,240Pu activity in soil samples was developed. The algorithm was tested during a radiological field survey of abandoned lands in Narodychi district. The results of the approbation showed a satisfactory convergence of obtained estimates of soil contamination with plutonium isotopes of Chernobyl origin with experimental results. The proposed algorithm may be a part of the decision-making system at reviewing the boundaries of radioactive contamination zones and returning in the use agricultural lands that were abandoned after the Chernobyl accident.
References
Radiological status of territories assigned to areas of radioactive contamination (in terms of districts) / K .: Ministry of Ukraine for Emergencies and Protection of the Population from the Consequences of the Chornobyl Catastrophe of Ukraine, 2008. 49 p.
The experience of overcoming the consequences of the Chernobyl disaster (agriculture and forestry) / P.P. Nadtochiy and others; K .: "World", 2003. 372 p.
Law of Ukraine "On the legal regime of the territory affected by radioactive contamination as a result of the Chernobyl disaster" of 27.02.91 № 791a-XII.- Information of the Verkhovna Rada of the USSR (VVR), 1991, № 16, p.198, https : //zakon.rada.gov.ua/laws/show/791%D0%B0-127.
Khomutinin Yu., Fesenko S., Levchuk S., Zhebrovska K., Kashparov V. (2020). Optimising sampling strategies for emergency response: Soil sampling. Journal of Environmental Radioactivity. 222, 106344 https://doi.org/10.1016/j.jenvrad.2020.106344
Kashparov V.A., Lundin S.M., Zvarich S.I., Yoschenko V.I., Levchuk S.E., Khomutinin Yu.V., Maloshtan I.N., Protsak V.P. (2003). Territory contamination with the radionuclides representing the fuel component of Chernobyl fallout. The Science of the Total Environment. 317(1-3), 105-119. https://doi.org/10.1016/S0048-9697(03)00336-X
Kashparov V., Levchuk S., Zhurba M., Protsak V., Khomutinin Yu., Beresford N.A., Chaplow J.S. (2018). Spatial datasets of radionuclide contamination in the Ukrainian Chernobyl Exclusion Zone. Earth System Science Data (ESSD). 10, 339-353. https://doi.org/10.5194/essd-10-339-2018
Pavlotskaya F.I. (1997). Basic principles of radiochemical analysis of environmental objects and methods for determining radionuclides of strontium and transuranium elements. Journal of Analytical Chemistry. 52(2) 126.
DSTU ISO 18589-4: 2015 Measurement of radioactivity in the environment. Soil. Part 4. Measurement of plutonium isotopes (plutonium 238 and plutonium 239 + 240) by alpha spectrometry
Chetyrkin E.M., Kalikhan I.L. (1982). Probability and statistics. M.: Finance and statistics, 319 p..
Kashparov V., Levchuk S., Zhurba M., Protsak, V. Beresford, N.A., Chaplow J.S. (2020). Spatial radionuclide deposition data from the 60 km radial area around the Chernobyl Nuclear Power Plant: results from a sampling survey in 1987. Earth System Science Data (ESSD). 12, 1861–1875, https://doi.org/10.5194/essd-12-1861-2020
Perkins R.W., Thomas C.W. (1980). Worldwide fallout. In Transuranic elements in the Environment: Tech. Inf. Center US Department of Energy: DOE/TIC_22880 / ed. W.C. Hanson. Washington, D.C. P. 53–82.
UNSCEAR Report to the General Assembly of Unated Nations with Annexes. – New York:UN, 1982. P. 228, p. 238.
Hemp E. F., Kudryashov V. P., Mironov V. P. (2006). Transuranium elements on the territory of Belarus. Minsk: Belarusian Science, 192 p.
Dufa C., Renaud P. (2005). 238Pu and 239+240Pu inventory and distribution through the lower Rhone valley terrestrial environment (Southern France). Science of the Total Environment. V. 348. P. 164–172
Michel H., Gasparro J., Barci_Funel G., Dalmasso J., Ardisson G., Sharovarov G. (1999). Radioanalytical determination of actinides and fission products in Belarus soils. Talanta. V. 48. P. 821–825.
Tobacco L.Ya. etc. (2002). Atlas Ukraine. Radioactive contamination. LLC "Intelligent GEO Systems". 2008.
Downloads
Published
Issue
Section
License
Relationship between right holders and users shall be governed by the terms of the license Creative Commons Attribution – non-commercial – Distribution On Same Conditions 4.0 international (CC BY-NC-SA 4.0):https://creativecommons.org/licenses/by-nc-sa/4.0/deed.uk
Authors who publish with this journal agree to the following terms:
- Authors retain copyright and grant the journal right of first publication with the work simultaneously licensed under a Creative Commons Attribution License that allows others to share the work with an acknowledgement of the work's authorship and initial publication in this journal.
- Authors are able to enter into separate, additional contractual arrangements for the non-exclusive distribution of the journal's published version of the work (e.g., post it to an institutional repository or publish it in a book), with an acknowledgement of its initial publication in this journal.
- Authors are permitted and encouraged to post their work online (e.g., in institutional repositories or on their website) prior to and during the submission process, as it can lead to productive exchanges, as well as earlier and greater citation of published work (See The Effect of Open Access).